Abstract
The coupling between electrical, thermal, and spin transport results in a plethora of novel transport phenomena. However, disentangling different effects is experimentally very challenging. We demonstrate that bilayers consisting of the antiferromagnetic insulator hematite (alpha-Fe2O3) and Pt allow one to precisely measure the transverse spin Nernst magnetothermopower (TSNM) and observe the low-temperature suppression of the platinum (Pt) spin Nernst angle. We show that the observed signal stems from the interplay between the interfacial spin accumulation in Pt originating from the spin Nernst effect and the orientation of the Neel vector of alpha-Fe2O3, rather than its net magnetization. Since the latter is negligible in an antiferromagnet, our device is superior to ferromagnetic structures, allowing one to unambiguously distinguish the TSNM from thermally excited magnon transport, which usually dominates in ferri/ferromagnets due to their nonzero magnetization. Evaluating the temperature dependence of the effect, we observe a vanishing TSNM below similar to 100 K. We compare these results with theoretical calculations of the temperature-dependent spin Nernst conductivity and find excellent agreement. This provides evidence for a vanishing spin Nernst angle of Pt at low temperatures and the dominance of extrinsic contributions to the spin Nernst effect.
Item Type: | Journal article |
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Faculties: | Chemistry and Pharmacy > Department of Chemistry |
Subjects: | 500 Science > 540 Chemistry |
ISSN: | 2469-9950 |
Language: | English |
Item ID: | 103086 |
Date Deposited: | 05. Jun 2023, 15:42 |
Last Modified: | 05. Jun 2023, 15:42 |