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Krok, Patrizia; Kozma, Ida Z.; Breuer, M.; Lochbrunner, Stefan; Riedle, Eberhard ORCID: 0000-0002-2672-5718 (2007): Search for pure vibrational dephasing of electronically excited dye molecules in solution. Frontiers in Optics 2007, 16–20 September 2007, San Jose, California, United States.
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Abstract

10 fs pulses compressed with Brewster-angled chirped mirrors are used to measure the vibronic wavepacket motion in a perylene dye. The coherence lifetime of 1.0 - 1.5 ps indicates that vibrational relaxation and pure dephasing contribute equally.