Uniaxial transition dipole moments in semiconductor quantum rings caused by broken rotational symmetry

Hartmann, Nicolai F.; Otten, Matthew; Fedin, Igor; Talapin, Dmitri; Cygorek, Moritz; Hawrylak, Pawel; Korkusinski, Marek; Gray, Stephen; Hartschuh, Achim und Ma, Xuedan (2019): Uniaxial transition dipole moments in semiconductor quantum rings caused by broken rotational symmetry. In: Nature Communications, Bd. 10, 3253

Abstract

Semiconductor quantum rings are topological structures that support fascinating phenomena such as the Aharonov-Bohm effect and persistent current, which are of high relevance in the research of quantum information devices. The annular shape of quantum rings distinguishes them from other low-dimensional materials, and enables topologically induced properties such as geometry-dependent spin manipulation and emission. While optical transition dipole moments (TDMs) in zero to two-dimensional optical emitters have been well investigated, those in quantum rings remain obscure despite their utmost relevance to the quantum photonic applications of quantum rings. Here, we study the dimensionality and orientation of TDMs in CdSe quantum rings. In contrast to those in other two-dimensional optical emitters, we find that TDMs in CdSe quantum rings show a peculiar in-plane linear distribution. Our theoretical modeling reveals that this uniaxial TDM originates from broken rotational symmetry in the quantum ring geometries.

• Dokumententyp: Zeitschriftenartikel
• Fakultät: Chemie und Pharmazie > Department Chemie
• Fakultätsübergreifende Einrichtungen: Center for NanoScience (CENS)
• Themengebiete: 500 Naturwissenschaften und Mathematik > 540 Chemie ; 500 Naturwissenschaften und Mathematik > 500 Naturwissenschaften
• ISSN: 2041-1723
• Sprache: Englisch